KnE Energy | VII International Conference on Photonics and Information Optics (PhIO) | pages: 38–46

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1. Introduction

Ultrafast lasers are used in various fields of science, engineering and medicine. Waveguides, optoelectronic systems, microchannels, laboratory on a chip are successfully created with the help of femtosecond (fs) lasers, and technological operations such as precision laser cutting, scribing, drilling and some others are carried out using powerful picosecond lasers. In addition, ultrafast lasers are an integral part of modern ophthalmology, for example, in corneal curvature correction [1] and cataract surgery [2,3]. High radiation intensity, as well as the universality of radiation absorption processes in transparent materials, are the reasons for the versatile application of ultrashort laser radiation. Ultrafast lasers can successfully perform micro-and nano-processing of polymers, glasses, fused quartz, as well as crystals, transparent ceramics and some other materials.

The advantage of using ultrafast lasers in these applications is the almost complete absence of thermal damage in the vicinity of the machined regions [4,5]. The reason for this is the nonlinear radiation absorption process, which is possible due to the ultra-short pulse duration. Therefore, the optical excitation of the electronic subsystem is terminated before the electron energy is transferred to the lattice.

Considerable attention has been paid to the investigation of the micromodifications formation, which are elongated in the direction of fs laser pulses propagation. The possibility of controlled formation of elongated micromodifications is promising tool for high-speed cutting and drilling of transparent dielectrics. Currently, several techniques are used to form elongated microcavities (Figure 1), for example, the use of Bessel beams [6], Kerr filamentation [7], interface spherical aberration (ISA) [8], diffraction effects [9].

The aim of the work is an experimental comparison of the methods for interaction region elongation of single fs laser pulses with the volume of transparent materials.

Figure 1

Scheme of formation of elongated micromodifications using different methods of lengthening the focal volume.

fig-1.jpg

2. Materials and Methods

Fig. 2 shows the scheme of the experimental setup. We used a femtosecond regenerative Yb laser (Avesta Project, RYF-10/35) to generate femtosecond pulses at a wavelength of 1025 nm, with pulse duration of 350 fs, pulse energy up to 150 μJ and repetition rate of 2000 Hz. Pulse picker based on the Pockels cell is built into the laser.

Figure 2

Experimental setup.

fig-2.jpg

We used the half-wave plate and the polarizer to control the energy. If necessary, the laser beam could be expanded by the LINOS (VIS-YAG 4X) beam expander. We used the following focusing systems: the Leitz Wetzlar objective, PLAN L50x, NA = 0.6; Lomo x10 objective NA = 0.1 and a high aberrated spherical lens with NA = 0.58. The lens was mounted on the z-translator, to control the focusing depth the radiation in the sample. The laser beam focused into a sample mounted on the x-y translator (Standa, 8MT173-50, 1 ÷ 800 μm / s and Newport, UTS50SS, 1 ÷ 40000 μm / s). The entrance surface of the sample was perpendicular to the beam. The average laser power was measured by a PD300-1W (350-1100 nm) sensor and a Nova meter (Ophir Photonics).

Polycarbonate plates (PC) with dimensions 3 x 20 x 50 mm were used as samples. The results of the action of focused fs pulses on the sample were recorded with a NIKON LV100D microscope.

The following experiment was carried out, to determine the differences in the spatial and structural modifications of the PCs formed in the samples using different focusing systems. Femtosecond laser pulses with a repetition rate of 100 Hz were focused through the entrance surface to the lower surface of the sample, then the sample moved along the X coordinate (Vx = 565.7 μm / sec) and the lens moved to the top (Vz = 565.7 μm / sec) which led to a shift of the focal region to the entrance surface. The use of this technique made it possible to observe the structural changes created per one FS impulse, depending on the focusing depth. In other experiments, the sample was processed at a constant focusing depth.

3. Results

Figure 3

Photographs of linear microstructures obtained by polycarbonate micromachining with single femtosecond pulses. a) NA = 0.1, E pulse = 10 μJ, F = 100 Hz, focusing depth 1 mm; b) Spherical lens, NA = 0.58, E pulse = 60 μJ, F = 100 Hz; c) NA = 0.6, E pulse = 8 μJ, F = 100 Hz, focusing depth 1 mm.

fig-3.jpg

Focusing of fs laser pulses in the bulk of polycarbonate using focusing optics with NA = 0.1 creates the necessary conditions for self-focusing and radiation filamentation, and as a result of the formation of elongated micromodifiсations with a length of more than 100 μm and a cross-sectional diameter about 2 μm. Results of the action of fs laser pulses with an energy of 10 μJ in the form of linear tracks of equal length are presented at Fig. 3 a). Laser scanning was performed only along the X coordinate at a speed of 800 μm / sec. Dependence of the length of tracks on the focusing depth is not observed.

In the case of using of spherical lens with NA = 0.58 and strong spherical aberrations as a focusing system, the volume modification has a complex spatial structure. The corresponding picture is shown in Fig. 3 (b). The scanning was simultaneously performed on the X and Z coordinates at 565.7 μm / sec. It is established that a single femtosecond pulse creates a linear structure in the sample along the radiation propagation axis, consisting of a sequence of filamentary micromodifications. These micromodifications are separated by regions with a modified refractive index. The total length (Σ) of the modified region exceeds 1000 μm. The dependence of the length of the modified region on the focusing depth is not observed. The line in the left part of the photo corresponds to the sample standing point ( 500 pulses). Increasing the of the laser pulse energy to 150 μJ leads to association of micromodifications in one Fig. 4.

Figure 4

Photograph of filamentary micromodifications created by single fs laser pulses in the volume of PC samples. The fs pulses are focused by a spherical lens with NA = 0.58. E pulse = 150 μJ, the focusing depth is constant.

fig-4.jpg

In the case of using objective (NA=0.6) instead of a spherical lens, whilemaintaining the other parameters of the system, FS pulse creates in a bulk only one micromodification that elongated on axis of radiation propagation (Fig. 3 c). In addition, it was found that increasing the focusing depth leads to an increase of the micromodification length, this corresponds to [10] and is explained by ISA at the air-sample boarder [11]. A change in the energy of the pulse leads to a decrease in the length of the filamentary micromodifications.

4. Discussion of results

The short duration of femtosecond pulses allows to reach the high peak powers, as well as an incredible intensity in the focal volume, which in turn can lead to nonlinear interactions with the material [12]. At the same time, it is known that the fs pulses focused in the sample volume can cause various modifications of the material structure: complete destruction of the material in the focal volume region, depolymerization, increase in the density of matter, graphitization and other [13,14], which causes a change in the optical and electrical characteristics of the material. The nature of the modifications depends on a number of parameters: the energy of the pulse, its duration, the characteristics of the energy distribution in the cross section of the beam, the depth of focusing, the scanning speed, and the properties of the material. The propagation of pulses with a high peak power can lead to Kerr's self-focusing, and as a consequence, to the collapse of the laser beam and filamentation. The formation of a laser filament in a volume of transparent dielectrics, together with a high intensity, leads to the formation of micromodification elongated in the direction of propagation (Fig. 1). To achieve the conditions of stable filamentation of femtosecond pulses in transparent materials, it is necessary to exceed the peak power of the pulse P above the critical power P cr .

It is known [12,15] that in the process of self-focusing, if the current power on the time profile of the ultrashort pulse exceeds the so-called critical power Pcr, then the laser beam begins to focus, and the position of the nonlinear focus (the focusing length) is determined by the Marburger formula:

znf=0.367ka2PpulsePcr1/20.85220.02191/2
Pcr=λ22πn0n2

where a is the radius of the laser beam at the entrance of the medium, k is the wave vector, Ppulse is the maximum peak input power, Pcr is the critical self-focusing power, n 0 is the linear refractive index, and n 2 is the nonlinear refractive index. If   we   pass the   laser   beam   through   a   focusing lens at the entrance surface of the medium, the focusing spot inside the medium shifts from the geometric focus towards the objective to a new position, which determined by the ratio    Ppulse/Pcr . The expression that determines the distance of displacement of the focusing spot from the position of the geometric focus f d with respect to the Marburger formula in this case has the form:

δ=fd2fd+znf.

Thus, it is clear that the main parameter affecting on the micromodification length during filamentation of the fs laser pulse is the excess of the peak pulse power over the critical power, which is individual for different materials. It should also be noted that self-focusing is more responsible for the formation of filamentary micromodification before of the geometric focus [15].

In the case of focusing by optical systems with high numerical apertures designed to work in parallel beams, the form of micromodifications can be very different from the sphere, and acquire the appearance of filamentary thread elongated in the direction of radiation propagation. The main reason for increasing the aspect ratio is the interface spherical lens aberration (ISA). ISA at the air-sample boundary extends the waist region towards the propagation of radiation. The length of the waist beyond the geometric focus (f d ) is determined by the formula proposed in [1,11]:

Δ=fdn*n2NA21NA2n,

where n=n 2 /n 1 =n 2 , with n 1 =1, f d - focusing depth, NA- numerical aperture of the objective. It can be seen that Δ (the length of the focal volume) is most sensitive to a change in the focusing depth (Δ f d ), the numerical aperture NA and indirectly to the energy of the pulse E pulse through a change in the energy at the peripheral rays in the energy distribution along the beam cross section.

The results (focusing of radiation with an objective with correction of spherical aberrations) of the increase in filament length with increasing focusing depth is in good agreement with the formula determining Δ.

Using a spherical lens as a focusing system leads to the formation of structures in the bulk of the sample that are significantly different from previous cases. Sequence of filamentary micromodifications with constant diameter (Figure 3b), arranged in succession along the propagation axis of fs laser pulse (z-axis) is formed. The length of the micromodifications in this sequence decreases towards the lens. The micromodifications are combined into a single and forming a microstructure 2 μm in diameter with an aspect ratio of more than 1000 (Fig. 4) with increasing pulse energy. The reason responsible for the formation of micromodifications of the presented spatial configuration is the transformation of the initial Gaussian distribution of laser radiation intensity into a set of diffraction ring of the Fresnel type. In this case, each diffraction ring has its own geometrical focus position, i.e. each diffraction ring will be focused in the air and in the material at different depths [9].

5. Conclusion

In this paper, the results of using various methods of extending the interaction region of single fs laser pulses with the volume of transparent materials were shown. The use of linear and nonlinear methods of lengthening the focal volume can become a promising tool for increasing productivity and quality in cutting and drilling of transparent materials with fs laser pulses. It is shown that the focusing of fs pulses into the bulk of polycarbonate by objective with a small numerical aperture can lead to self-focusing, and as a consequence to the formation of an extended filamentary micromodification. In this case, the length of the micromodification does not depend on the focusing depth, and is determined by the peak power of the laser pulse. In the case of high numericaql aperture lenses, the micromodification region formed by a single fs pulse in the sample volume can be very different from the sphere and have the form of thread whose length depends on the focusing depth and the numerical aperture and is determined by the interface spherical aberration. When using a spherical lens with a large numerical aperture and strong spherical aberrations as a focusing system, a sequence of micromodifications located along the optical axis is formed in the volume of the sample under the action of a single femtosecond pulse. The total length of the modified region depends on the energy of the laser pulse and can exceed 1 mm. The dependence of the micromodification length on the focusing depth is not observed.

Acknowledgements

This work was partially supported by Foundation for Assistance to Small Innovative Enterprises inScience and Technology, program U.M.N.I.K. (10624GU/2016 No. 0023590).

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